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In article number 1806562, Lin Wang, Wei Huang, and co‐workers describe the synthesis of PbI2 with a unique electronic structure down to the atomic scale by a solution method, and construct versatile interfacial semiconductors via band alignment engineering. As an illustrative example, MoS2, WS2, and WSe2 monolayers show completely distinct light–matter interactions when interfacing with PbI2, which...
To explore new constituents in two‐dimensional (2D) materials and to combine their best in van der Waals heterostructures is in great demand as being a unique platform to discover new physical phenomena and to design novel functionalities in interface‐based devices. Herein, PbI2 crystals as thin as a few layers are synthesized, particularly through a facile low‐temperature solution approach with crystals...
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