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Main‐group element indium (In) is a promising electrocatalyst which triggers CO2 reduction to formate, while the high overpotential and low Faradaic efficiency (FE) hinder its practical application. Herein, we rationally design a new In single‐atom catalyst containing exclusive isolated Inδ+–N4 atomic interface sites for CO2 electroreduction to formate with high efficiency. This catalyst exhibits...
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