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Protonated achiral H2TPPS4 spontaneously self‐arranges at acids pH and high ionic strength to build mesoscopic J‐aggregates that are intrinsically chiral. According to the symmetry rule aggregation leads to a racemate that, however, can be unbalanced by chemical (chiral pollutants) or physical stimuli (as vortexing the solution). Vortexing the title racemate, in principle, might either induce chiral...