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A new series of RDT-EDO-TTF [R=C5, C6, C7, C8; (cis-l,2-cycloalkylene-l,2-dithio)ethylenedioxytetrathiafulvalene and R=Bz; (benzodithio)ethylenedioxytetrathiafulvalene] donors containing cycloalkylene or benzene, and ethylenedioxy groups as a source of the steric hindrance and the intermolecular hydrogen bonds has been synthesized. The charge transfer (CT) salts, β″-(RDT-EDO-TTF) 2 (PF ...
We have obtained several charge-transfer complexes of CnDTP-TTF (n=5,6). The C5DTP-TTF salts are the κ-type semiconductor with high room-temperature conductivities, whereas β′′-(C6DTP-TTF) 2 (GaCl 4 ) 0.66 shows the metallic behavior down to 40K. In order to improve the conductivity by increasing the bandwidth, we have applied a pressure and synthesized a series of the selenium...
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