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High frequency (GHz) signals are sent to a scanning tunneling microscope probe down to the surface of an alkylferrocene self‐assembled monolayer in liquid and allow to measure locally electrochemical charge transfer corresponding to currents on the order of attoampere. This technique, presented in article number 2101253 by Nicolas Clément, Georg Gramse, and co‐workers, opens the way to unprecedented...
Electrochemical microscopy techniques have extended the understanding of surface chemistry to the micrometer and even sub‐micrometer level. However, fundamental questions related to charge transport at the solid‐electrolyte interface, such as catalytic reactions or operation of individual ion channels, require improved spatial resolutions down to the nanoscale. A prerequisite for single‐molecule electrochemical...
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