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Plasma treatment and reduction are used to synthesize Pt nanoparticles (NPs) on nitrogen‐doped carbon nanotubes (p‐Pt/p‐NCNT) with a low Pt content. In particular, the plasma treatment is used to treat the NCNT to give it with more surface defects, facilitating a better growth of the Pt NPs, while the plasma reduction produces the Pt NPs with a reduced fraction of the surface atoms at the high oxidation...