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A porous actuator is prepared using a liquid crystal elastomer (LCE) loaded with metal‐organic framework (MOF) nanoparticles (MIL‐88A). While the swellable MOF additive endows the LCE actuator with nanoscale pores, after its removal by chemical etching, macroporous LCE actuator is obtained. This LCE‐MOF actuator displays several interesting features. 1) Selective etching allows the actuator in water...