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The artificial solid electrolyte interphase (SEI) plays a pivotal role in Zn anode stabilization but its long‐term effectiveness at high rates is still challenged. Herein, to achieve superior long‐life and high‐rate Zn anode, an exquisite electrolyte additive, lithium bis(oxalate)borate (LiBOB), is proposed to in situ derive a highly Zn2+‐conductive SEI and to dynamically patrol its cycling‐initiated...
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