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The Pt-catalysed oxidation of the alcohol methyl α-D-glucopyranoside to 1-O-methyl α-D-glucuronic acid has been studied under varying pH conditions. Two types of catalysts with different metal dispersion are used, that is, Pt on active carbon support and Pt on graphite support. The pH of the reaction medium is varied between 6 and 10. The initial reaction rate increases with an increase in pH, and...
A reaction-engineering model is presented, which describes catalyst performance as a function of the catalyst activity profile, the reaction kinetics, and the degree of catalyst deactivation. With this model, the catalyst activity profile can be optimised for Pt catalysed methyl α-d-glucopyranoside (slowly-reactive) and glucose (highly-reactive) oxidations. This is done by comparing modelling results...
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