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Can the active kernels in ultrasmall metal nanoparticles (nanoclusters, NCs) react with one another, or can the internanocluster reaction occur when they are in close enough proximity? To resolve this fundamental issue, we investigated the solid‐state internanocluster reaction of the most studied gold NC Au25(SR)18 (SR: thiolate). A novel NC was produced by increasing the pressure to 5 GPa, whose...
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