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In this study we investigate the pyramidalization of the sp2‐hybridized center at the ipso‐carbon atom Ci of phenyl compounds on the theoretical side by DFT calculations of toluene, t‐butylbenzene, and ethylbenzene and on the experimental side by a scatter plot analysis of 14,169 structures of ethylbenzene compounds Cβ−CαH2−C6H5 with three open positions for variation at Cβ, accumulated in the Cambridge...
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