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Capturing the microscopic motion of an individual molecule on the femtosecond time scale with atomic spatial resolution has remained a key open challenge of modern nanoscience. Here, we bring the concept of lightwave-driven sub-cycle charge transport, the paradigm underlying high-harmonic generation, to a new arena of atomic spatial resolution. We enter an unprecedented regime of ultrafast lightwave-driven...
Field-resolved detection of ultrafast pulses in the THz (0.1–10 THz) and multi-THz (10–100 THz) spectral range has provided key insights into the dynamics of low-energy collective excitations in condensed matter systems. However, the spatial resolution of these far-field studies is intrinsically limited to the scale of the probing wavelength by diffraction. Thus, the measured optical response is an...
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