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Actinyl chemistry is extended beyond Cm to BkO2+ and CfO2+ through transfer of an O atom from NO2 to BkO+ or CfO+, establishing a surprisingly high lower limit of 73 kcal mol−1 for the dissociation energies, D[O‐(BkO+)] and D[O‐(CfO+)]. CCSD(T) computations are in accord with the observed reactions, and characterize the newly observed dioxide ions as linear pentavalent actinyls; these being the first...
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