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The interplay between the electronic structure and reconstruction of the geometry on a surface is an intriguing and exciting investigation. One classic example that has been one of the first systems to be identified using the angularly resolved photo-emission spectroscopy and scanning tunnelling microscopy is the Herringbone reconstruction on the Au(111) surface. Here, we report on the results derived...
In this perspective we discuss how an intimate interaction of experiments with theory is able to deepen our insight into the catalytic reaction system on the molecular level. This strategy is illustrated by discussing various examples from our own research of surface chemistry and model catalysis. The particular examples were carefully chosen to balance the specific strength of both approaches – theory...
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