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Imaging photoelectron photoion coincidence (iPEPICO) spectroscopy has been used to determine 0K appearance energies for the unimolecular dissociation reactions of several energy selected straight chain alkyl iodide cations 1-CnH2n+1I+→CnH2n+1++I, (n=3–7). The 0K appearance energy of iodine atom loss, yielding in fact the 2-alkyl radical cation up to n=6, was determined to be 9.836±0.010, 9.752±0.010,...
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