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Our recent studies of the steady-state kinetics of the N 2 O–CO reaction on Rh(110) indicate that at CO excess, the reaction rate increases with increasing temperature. At N 2 O excess, the reaction rate is nearly independent of temperature at T<520K and rapidly decreases with increasing temperature at T>520K. Our present analysis of the relevant data indicates that the latter...
Under temperature-programmed conditions, N 2 O decomposition occurs on Rh(110) between 60 and 190K and results in N 2 desorption. Experimental studies of the angular distribution of the flux of the reaction products indicate that N 2 molecules leave the surface both during and after N 2 O dissociation events. The N 2 TPD spectra observed are complex. In particular,...
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