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Perylenediimides (PDIs) and perylenemonoimide diesters (PMIs) can be selectively substituted at the 1,6‐ or 7,12‐ positions of the bay region, respectively, by direct amination reactions. The reactions proceed by the formation of a perylene radical anion and its subsequent oxidation, and the yields range from 20–97 %. The amination can be tuned to obtain either mono‐ or disubstituted perylenes by...
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