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The cationic allylpalladium complexes 3a–3f, 4a, 4e, 5e of type [Pd(η3‐2‐Me‐C3H4)P2]PF6 were synthesized using a group of monodentate P‐stereogenic phosphanes, P=PPhRR′ (a–f) and diphosphanes (PhRPCH2)2 (1a, 1e) or PhRPCH2Si(Me)2CH2PPhR (2e). The analogous cationic complexes with the disubstituted allyl group (η3‐1,3‐Ph2‐C3H3) and monodentate phosphanes were not isolated as stable solids; only [PdCl(η...
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