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Single crystal X-ray diffraction reveals that 4,4′-bis(tetrahydrothiopyranyl) crystallizes in an equatorial–equatorial geometry with a gauche conformation along the central carbon–carbon bond. B3LYP/6-311G ** and MP2/6-311G ** calculations show that the antiperiplanar conformation is higher in energy than the gauche one because of sulfur induced stretching and widening of the cyclohexane-like...
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