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The visible light‐promoted intramolecular [2+2] cycloaddition of N‐allylcinnamamines and N‐allylcinnamamides in the presence of catalytic amounts of [Ir{dF(CF3)ppy}2(dtbpy)]PF6 is reported. Low energy visible light and a high triplet energy iridium‐photosensitizer were efficient at promoting the cycloaddition reaction of N‐allylcinnamamides and N‐allylcinnamamines to the corresponding aryl‐3‐azabicyclo[3...
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