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Elektrochemische radikalische Polymerisation ermöglicht das Züchten von Ruthenium(II)‐Vinylpolypyridyl‐Komplexen in den Hohlräumen von TiO2‐Filmen, wie T. J. Meyer et al. in der Zuschrift auf S. 4972 ff. beschreiben. Der so erhaltene Film hat Potenzial für die Lichtumwandlung in Farbstoffsolar‐ und Photoelektrosynthesezellen, die in wässriger Umgebung betrieben werden.
Surface‐initiated, oligomeric assemblies of ruthenium(II) vinylpolypyridyl complexes have been grown within the cavities of mesoporous nanoparticle films of TiO2 by electrochemically controlled radical polymerization. Surface growth was monitored by cyclic voltammetry as well as UV/Vis and X‐ray photoelectron spectroscopy. Polymerization occurs by a radical chain mechanism following cyclic voltammetry...
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