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Light‐driven water splitting was achieved using a dye‐sensitized mesoporous oxide film and the oxidation of bromide (Br−) to bromine (Br2) or tribromide (Br3−). The chemical oxidant (Br2 or Br3−) is formed during illumination at the photoanode and used as a sacrificial oxidant to drive a water oxidation catalyst (WOC), here demonstrated using [Ru(bda)(pic)2], (1; pic=picoline, bda=2,2′‐bipyridine‐6,6′‐dicarboxylate)...
The use of electropolymerization to prepare electrocatalytically and photocatalytically active electrodes for water oxidation is described. Electropolymerization of the catalyst RuII(bda)(4‐vinylpyridine)2 (bda=2,2′‐bipyridine‐6,6′‐dicarboxylate) on planar electrodes results in films containing semirigid polymer networks. In these films there is a change in the water oxidation mechanism compared to...
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