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The synthesis, structural, photophysical, theoretical, and electrochemical characterization of four tris(2‐phenylpyridine)‐based IrIII complexes are reported. The complexes were functionalized on the pyridine or on the phenyl rings with amide moieties substituted with a tris(ethyl)amine or ethyl groups, thereby yielding a family of compounds with hemicaged or open (without a capping unit but with...
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