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The recognition of the dual binding mode of propargyl and allyl alcohols to [Cp*Ru] fragments fostered the development of a highly regioselective intermolecular Alder‐ene‐type reaction of alkynes with 1,2‐disubstituted alkenes. The increased substrate scope opens new perspectives in stereochemical terms. As the loaded catalyst is chiral‐at‐metal, stereochemical information is efficiently relayed from...
Deformationsverbot: Für Adenin in (dA)10 wird die innere Konversion zum Grundzustand durch eine konische S0/S1‐Überschneidung mit stark aus der Ebene herausgedrehter Aminogruppe bestimmt (links). In (dA)10⋅(dT)10 wird dieser Pfad durch die Bildung von Adenin‐Thymin‐Wasserstoffbrücken unterbunden (rechts). Für angeregtes Adenin in DNA‐Strängen werden zehnmal längere Lebensdauern berechnet als im Vakuum...
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