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Oxidative halogenation with trityl chloride provides convenient access to CeIV and UIV chloroamides [M(N{SiMe3}2)3Cl] and their N‐heterocyclic carbene derivatives, [M(L)(N{SiMe3}2)2Cl] (L=OCMe2CH2(CNCH2CH2NDipp) Dipp=2,6‐iPr2C6H3). Computational analysis of the bonding in these and a fluoro analogue, [U(L)(N{SiMe3}2)2F], provides new information on the covalency in this relative rare oxidation state...
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