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Catalytic reactions via the cleavage of two classes of unstrained carbon–carbon bonds are reviewed. One is the carbon–acyl bond in ketones, which can be activated via oxidative addition, with the aid of a directing group in most cases. The other is the carbon–cyano bond in nitriles, which can be activated via oxidative addition or a silicon‐ or boron‐assisted two‐step mechanism. In addition to the...
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