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On page 5946, Tobin J. Marks, Mark A. Ratner, Michael T. Lanagan, and co‐workers report a series of metal oxide core/Al2O3 shell polypropylene nanocomposites synthesized via in situ polymerization utilizing a metallocene polymerization catalyst chemisorbed on the nanoparticle surfaces. The good particle dispersion and tunable shell thickness afford materials with high energy storage capacities and...
Dielectric loss in metal oxide core/Al2O3 shell polypropylene nanocomposites scales with the particle surface area. By moderating the interfacial surface area between the phases and using increasing shell thicknesses, dielectric loss is significantly reduced, and thus the energy stored within, and recoverable from, capacitors fabricated from these materials is significantly increased, to as high as...
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