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The 1H NMR spectroscopic analysis of the binding of the ClO4− anion to the hydrophobic, concave binding site of a deep‐cavity cavitand is presented. The strength of association between the host and the ClO4− anion is controlled by both the nature and concentration of co‐salts in a manner that follows the Hofmeister series. A model that partitions this trend into the competitive binding of the co‐salt...
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