On one hand electron or hole doping of quantum spin liquid (QSL) may unlock high‐temperature superconductivity and on the other hand it can disrupt the spin liquidity, giving rise to a magnetically ordered ground state. Recently, a 2D MOF, Cu
3(HHTP)
2 (HHTP ‐ 2,3,6,7,10,11‐hexahydroxytriphenylene), containing Cu(II) S=
frustrated spins in the Kagome lattice is emerging as a promising...