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Cation–cation interaction: A new 2 D sheet structure containing a side‐on cation–cation interaction (CCI) has been synthesized and characterized (see figure). Unprecedentedly, no chelating ligands between the cations are present. The nature of the side‐on interaction and ligand effects has been explored by using a variety of quantum chemical methods. The spin–orbit‐coupled ground state mixes singlet,...
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