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During the last decade, the chemistry of d0/fn actinides hasflourished reaching a high level of sophistication. Compared to the early or late transition-metalcomplexes and lanthanides, the actinides sometimes exhibit parallel but mostly complementary activitiesfor similar organic processes, and sometimes even challenge the activities of the transition...
The reaction of one equivalent of Cp* 2 UCl 2 with 2-(trimethylsilylimino)-1,3-di-tert-butylimidazoline in boiling toluene afforded a one electron oxidation of the uranium metal and the opening of the N-heterocyclic ring, resulting in the formation of an organometallic uranium(V) imine complex. This complex crystallized with one molecule of toluene in the unit cell, and its solid-state...
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