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Changes in pH have been used to shift the band-edge positions of n-type ZnO electrodes relative to solution-based electron acceptors having pH-independent redox potentials. Differential capacitance vs. potential and current density vs. potential measurements using [Co(bpy) 3 ] 3+/2+ and [Ru(bpy) 2 (MeIm) 2 ] 3+/2+ (where bpy=2,2′-bipyridyl and MeIm=1-methyl-imidazole)...
Optically induced charge transfer between adsorbed molecules and a metal electrode was predicted by Hush to lead to new electronic absorption features, but has been only rarely observed experimentally. Interfacial charge transfer absorption (IFCTA) provides information concerning the barriers to charge transfer between molecules and the metal/semiconductor and the magnitude of the electronic coupling...
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