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Der (cAAC)2Mn‐Komplex (cAAC=cyclisches Alkyl(amino)carben) enthält ein lineares zweifach koordiniertes Mn‐Zentrum. Die antiferromagnetische Wechselwirkung eines ungepaarten Elektrons, das zwischen den zwei Carben‐C‐Atomen delokalisiert ist, mit dem zentralen MnI, das eine d6‐Konfiguration hat, trägt hauptsächlich zum ST=3/2‐Grundzustand bei. Die Behandlung von (cAAC)2Mn mit H2 bei Raumtemperatur führt...
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