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Two di‐tert‐butylphenols incorporating an N‐methylbenzimidazole moiety in the ortho or para position have been synthesised (MeOH and pMeOH, respectively). Their X‐ray structures evidence a hydrogen bond between the phenolic proton and the iminic nitrogen atom, whose nature is intra‐ and intermolecular, respectively. The present studies demonstrate that MeOH is readily oxidised by an intramolecular...
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