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Herein, we communicate a selective and efficient protocol for oxidative arylating carbocyclization of enallenynes using O2 as the oxidant. The key to success for this aerobic transformation is the application of a specific electron transfer mediator (ETM), a bifunctional catalyst consisting of a metal‐macrocycle and quinone moieties. This catalyst significantly facilitates the reoxidation of Pd0 to...
Kein Druck: Die Oxidation aromatischer C‐H‐Bindungen bei Raumtemperatur gelingt durch eine kupferkatalysierte „Oxygenase‐artige“ Oxidation von Arenen und Heteroarenen in Gegenwart von Luft (siehe Schema). Die Reaktion umfasst einen Sauerstoffatomtransfer vom O2 der Luft auf das Substrat.
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