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A binary catalyst of CaO–ZnO is effective for the selective conversion of CH 4 to C 2 hydrocarbons using CO 2 as the oxidant. C 2 selectivity approaches 80% with a C 2 yield of 4.3% over the catalyst with a Ca/Zn ratio of 0.5 at 875°C. The lattice oxygen of the CaO–ZnO converts CH 4 mainly to H 2 and CO. The presence of CO 2 forms a new...
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