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The magnetic properties of α-Cu(dca) 2 (pyz) were examined by magnetic susceptibility, magnetization, inelastic neutron scattering (INS), muon-spin relaxation (μSR) measurements and by first-principles density functional theoretical (DFT) calculations and quantum Monte Carlo (QMC) simulations. The χ versus T curve shows a broad maximum at 3.5K, and the data between 2 and 300K is well described...
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