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Here, an unidentified type of micropillar growth is described at room temperature during conventional direct‐current magnetron sputtering (DC‐MS) deposition from a Li4Ti5O12+graphite sputter target under negative substrate bias and high operating pressure. These fabricated carbon–Li2O–TiO2 microstructures consisting of various Li4Ti5O12/Li2TiO3/LixTiO2 crystalline phases are demonstrated as an anode...
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