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Recently, the development of more sustainable catalytic systems based on abundant first‐row metals, especially nickel, for cross‐coupling reactions has attracted significant interest. One of the key intermediates invoked in these reactions is a NiIII–alkyl species, but no such species that is part of a competent catalytic cycle has yet been isolated. Herein, we report a carbon–carbon cross‐coupling...
Mach′s Dir leicht: Eine Vielzahl an Ketonen und zwei Aldehyde wurden unter milden Bedingungen in Gegenwart des Titelkomplexes effizient hydrosilyliert (siehe Schema; R,R′=H, Alkyl, Aryl). In manchen Fällen genügten 0.01 bis 0.03 Mol‐% an Katalysator. Dieses Verfahren könnte sich als einfache, kostengünstige und umweltverträgliche Alternative zu den derzeitigen Methoden für die Hydrosilylierung von...
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