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A series of dangling chain based-polyurethane/poly(methyl methacrylate) (DPU/PMMA) filled with exfoliated layered double hydroxides (LDH) were synthesized by methyl methacrylate in-situ intercalative polymerization. The dangling chains were introduced by using vegetable oils as chain extender. The effect of dangling chain and the contents of LDH on the molecular dynamics of DPU/PMMA was investigated...
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