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In the search for multifunctional molecular materials, we designed an enantiopure pair of FeII complexes with chiral, chelating (R)/(S)‐4,5‐pinenepyridyl‐2‐pyrazine ligands exhibiting three inherent physical properties: chirality, spin crossover, and dielectric switching. The geometrical change resulted in coupling of the spin‐crossover transition at 187 K to dielectric switching. Both compounds were...
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