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The double phosphate Cs3In3(PO4)4, prepared by a flux technique, features a fragment of composition In3O16 formed by three corner‐sharing InO6 polyhedra. The central In atom resides on a twofold rotation axis, while the other two In atoms are on general positions. The O atoms in this fragment also belong to PO4 tetrahedra, which link the structure into an overall three‐dimensional anionic In–O–P network...
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