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Dimeric μ-oxo ions such as cis,cis-[(bpy) 2 Ru(OH 2 )] 2 O 4+ , its congeners containing ring-substituted bipryidine ligands, and related structures have long been known to efficiently catalyze water oxidation by strong chemical oxidants and at electrode surfaces. However, despite considerable effort, the goal of identifying the underlying molecular mechanisms has not...
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