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The magnetocrystalline anisotropy of a ferromagnet is determined by its crystal structure and is thus an inherent source of magnetic anisotropy.[1,2] It is the key to an understanding of ferromag-netism itself and is still actively investigated even for apparently well-understood materials such as Fe.[3-5] The magnetocrystalline anisotropy energy of bcc Fe can be expressed in terms of the direction...
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