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The [Fe(L222N5)(CN)2] compound, where L222N5 refers to the macrocyclic Schiff‐base ligand, 2,13‐dimethyl‐3,6,9,‐12,18‐pentaazabicyclo[12.3.1]octadeca‐1(18),2,12,14,‐ 16‐pentaene, is a photomagnetic FeII based coordination compound, which undergoes light‐induced excited spin‐state trapping (LIESST). The low spin state is hexacoordinated and the high spin state heptacoordinated. This system also serves...
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