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Inorganic CsSnI3 with low toxicity and a narrow bandgap is a promising photovoltaic material. However, the performance of CsSnI3 perovskite solar cells (PSCs) is much lower than that of Pb‐based and hybrid Sn‐based (e.g., CsPbX3 and CH(NH2)2SnX3) PSCs, which may be attributed to its poor film‐forming property and the deep traps induced by Sn4+. Here, a bifunctional additive carbazide (CBZ) is adapted...
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