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Precise morphology design and electronic structure regulation are critically significant to promote catalytic activity and stability for electrochemical hydrogen production at high current density. Herein, the carbon nanotube (CNT) encapsulated Fe‐doped NiCoP nanoparticles is in‐situ grown in hierarchical carbonized wood (NCF0.5P@CNT/CW) for water splitting. Coupling merits of porous carbonized wood...