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Boron, as a unique element nearest to carbon in the periodic table, has been predicted to form many distinctive two‐dimensional (2D) structures that significantly differ from other well‐studied 2D materials, owning to its exceptional ability to form strong covalent two‐center‐two‐electron bonds as well as stable electron‐deficient multi‐center‐two‐electron bonds. Until recently, the successful syntheses...
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