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Manipulating the backbone of small molecule acceptors (SMAs) is of particular importance in developing efficient organic solar cells (OSCs). The common design is constructing 2‐arm SMAs with linear or curved backbones. Herein, we report an acceptor 4A‐DFIC with a 4‐arm backbone unexpectedly generated in the reaction of an electron‐rich aromatic diamine and hexaketocyclohexane. Single‐crystal X‐ray...
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