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The infrared spectrum of the cross-shaped van der Waals complex CO2–CS2 is observed in the region of the CO2 ν3 fundamental band (≈2350cm−1) using a tuneable diode laser to probe a pulsed supersonic slit jet expansion. Two combination bands are assigned, corresponding to the intermolecular torsion and CO2 bend modes, and their positions and rotational structure agree extremely well (<0.1cm−1) with...
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